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High temperature ferromagnetic ordering in c-axis oriented ZnO:Mn nanoparticle thin films by tailoring substrate temperature
Citation
Usman Ilyas, Lee, P., Tan, T. L., Ramanujan, R. V., Zhang, S., Chen, R., Sun, H. D., & Rawat, R. S. (2014). High temperature ferromagnetic ordering in c-axis oriented ZnO: Mn nanoparticle thin films by tailoring substrate temperature. International Journal of Modern Physics: Conference Series, 32(2014), Article 1460341. https://doi.org/10.1142/S201019451460341X
Author
Usman Ilyas
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•
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Ramanujan, Raju V.
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Zhang, Sam
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Chen, R.
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Sun, H. D.
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Abstract
This study reports the enhanced ferromagnetic ordering in ZnO:Mn nanoparticle thin films, grown at different substrate temperatures using pulsed laser deposition. The optimum growth conditions were deduced from X-ray, photoemission and magnetic measurements. The X-ray measurements reveal that there was an optimum substrate temperature where the thin films showed relatively stronger texture, better crystallinity and lower strain. Substrate temperature tuned the deep level recombination centers in ZnO:Mn, which changed the optical quality by altering the electronic structure. The M-H curves, in the present study, revealed superior ferromagnetic response of 20-nm sized particles in ZnO:Mn thin film grown at a substrate temperature of 450 °C. Ferromagnetic ordering becomes weaker at higher/lower substrate temperatures due to the activation of native defects in ZnO host matrix.
Date Issued
2014
Publisher
World Scientific
Journal
International Journal of Modern Physics: Conference Series
DOI
10.1142/S201019451460341X